Evaluations of the mechanical and physical properties of galangal root-poly(butylene-succinate) (PBS)-based biocomposite
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Abstract
Various agricultural waste materials, such as cassava stems, pineapple leaves, banana peels, and corn pulp, were developed into natural biodegradable packaging, adding value to the agricultural waste. Hence, this research aimed to develop the biocomposites and inspect their mechanical and physical properties. Fresh galangal root waste was washed and dried at 80°C for 12 hours and then ground to achieve a particle size of 250 microns (GR250) and 400 microns (GR400). Then, they were mixed with PBS at the ratio of PBS: GR250 at 80:20 wt.%. Later, the mixtures were passed through the extruder, and the plastic strands were obtained. Later, these plastic strands were shredded into small pellets called biocomposite pellets. These pellets were formed by heat at 150°C for 5 minutes under a pressure of 10 MPa to obtain the biocomposite specimens. Then, they were assessed the mechanical properties (tensile strength, impact strength, and flexural strength). Also, the physical properties (water absorption, density, morphology, and percentage of natural degradation) were performed. The results could imply that adding GR250 and GR400 into PBS-based biocomposite could cause reductions in structural integrity and elasticity. PBS/GR biocomposites would assert less impact force. The results could reflect that PBS/GR250 and PBS/GR400 biocomposites had more ability to resist bending stresses than neat PBS. PBS/GR400 biocomposites tended to degrade faster, as supported by microstructure observation and lower density compared to PBS/GR250. It could be concluded that the galangal root waste could be added value by developing into a based-biocomposite. Galangal root waste can produce biocomposite food containers that can resist bending stresses. Biocomposite food containers have a natural biodegradable property and environmentally friendly aspects.
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References
Visakha Phuchinda. Monitoring and evaluation project to promote the reduction of single-use plastics. Complete report [Internet]. Department of Environmental Quality Promotion, Ministry of Natural Resources and Environment; 2023 [cited 2024 Jun 24]. Availability from: http://164.115.46.29/media/details?media_group_code=10&media_type_id=30&media_id=4903.
FAO. The State of Food and Agriculture 2019. Moving forward on food loss and waste reduction [Internet]. Food and Agriculture Organization of the United Nations; 2019 [cited 2023 Dec 12]. Availability from: https://www.fao.org/3/ca6030en/ca6030en.pdf.
Baranwal J, Barse B, Fais A, Delogu GL, Kumar A. Biopolymer: a sustainable material for food and medical applications. Polymers. 2022;14:983.
Rambabu K, Bharath G, Banat F, Show PL, Cocoletzi HH. Mango leaf extract incorporated chitosan antioxidant film for active food paGRaging. Int J Biol Macromol. 2019;126:1234-43.
de Moraes Crizel T, de Oliveira Rios A, Alves VD, Bandarra N, Moldão‐Martins M, Flôres SH. Active food paGRaging prepared with chitosan and olive pomace. Food Hydrocolloids. 2018;74:139-50.
Moudache M, Colon M, Nerín C, Zaidi F. Phenolic content and antioxidant activity of olive by-products and antioxidant film containing olive leaf extract. Food Chem. 2016;212:521-27.
Hanani ZAN, Husna ABA, Syahida SN, Nor-Khaizura MAB, Jamilah B. Effect of different fruit peels on the functional properties of gelatin/polyethylene bilayer films for active paGRaging. Food PaGRaging and Shelf Life. 2018;18:201-11.
Hanani ZAN, Yee FC, Nor-Khaizura MAR. Effect of pomegranate (Punica granatum L.) peel powder on the antioxidant and antimicrobial properties of fish gelatin films as active paGRaging. Food Hydrocolloids. 2019;89:253-59.
Zhao Y, Saldaña MDA. Use of potato by-products and gallic acid for development of bioactive film paGRaging by subcritical water technology. The Journal of Supercritical Fluids. 2019;143:97-106.
Riaz A, Lei S, Akhtar HMS, Wan P, Chen D, Jabbar S, et al. Preparation and characterization of chitosan-based antimicrobial active food paGRaging film incorporated with apple peel polyphenols. Int J of Bio Macromolecules. 2018;114: 547-55.
Priyadarshi R, Sauraj Kumar B, Deeba F, Kulshreshtha A, Negi YS. Chitosan films incorporated with Apricot (Prunus armeniaca) kernel essential oil as active food packaging material. Food Hydrocolloids. 2018;85:158-66.
Nor Adilah A, Jamilah B, Noranizan MA, Nur Hanani ZA. Utilization of mango peel extracts on the biodegradable films for active packaging. Food Packag Shelf Life. 2018;16:1-7.
Dilucia F, Lacivita V, Conte A, Nobile MAD. Sustainable use of fruit and vegetable by-products to enhance food packaging performance. Foods. 2020;9:857.
Peñas MI, Pérez-Camergo RA, Hernández R, Müller AJ. A Review on current strategies for the modulation of thermomechanical, barrier, and biodegradation properties of poly (butylene succinate) (PBS) and its random copolymers. Polymers. 2022;14:1025.
Office of Agricultural Economics, 2015. Polybutylene succinate (PBS) [Internet]. PACKAGING INDUSTRIAL INTELLIGENCE UNIT; [cited 2024 Nov 10]. Availability from: https://packaging.oie.go.th/new/admin_control_new/html-demo/file_technology/9480617235.pdf.
Jantana S, Jannok P, Nithikarnjanatharn J. Mechanical and Physical Properties of Poly (lactic acid)-Based Biocomposite Composed of Food Production Residue. In: World Integrated Chemical and Material Engineering Technology Conference 2023; Bangkok, Thailand. WICMETC; 2023.
Nithikarnjanatharn J, Samsalee N. Effect of cassava pulp on Physical, Mechanical, and biodegradable properties of Poly(Butylene-Succinate)-Based biocomposites. Alexandria Engineering Journal. 2022;61:10171-81.
Kha lueang : galangal [Internet]. Thailand: Department of Agricultural Extension. 2024 [cited 2024 Nov 10]. Availability from: http://www.agriman.doae.go.th/herbal/herbdoae005/kha%20lueang.pdf.
Liu L, Yu J, Cheng L, Qu W. Mechanical properties of poly(butylene succinate) (PBS) biocomposites reinforced with surface modified jute fiber. Composites: Part A. 2009;40:669-74.
Prasoetsopha N, Thainoi P, Jinnavat R, Charerntanom W, Hasook A, Singsang W. Morphological and Mechanical Properties of Natural Rubber Compound/Poly(butylene succinate) Blend. IOP Conf Ser Mater Sci Eng. 2020;840:012013.
Mochane MJ, Magagula SI, Sefadi SJ, Mokhena TC. A review on green composites based on natural fiber-reinforced polybutylene succinate (PBS). Polymers. 2021;13:21-38.
ASTM International (ASTM D638). Standard test method for tensile properties of plastics, in annual book of ASTM standards. West Conshohocken: ASTM International; 2022.
ASTM International (ASTM D256). Standard test methods for determining the Izod pendulum impact resistance of plastics, in annual book of ASTM standards, West Conshohocken: ASTM International; 2018.
ASTM International (ASTM D790. Standard test methods for flexural properties of unreinforced and reinforced plastics and electrical insulating materials, in annual book of ASTM standards. West Conshohocken: ASTM International; 2017.
ISO, Paper and board-Determination of water absorptiveness-Cobb method. 4th ed. International standard. 2023.
Suntudprom J, Phiaphumipong P, Jannok P, Meeklangsaen W, Sukthang N, Prangpru N, et al. Adding value to waste from corn cob for producing biocomposites. In the 14th Academic Conference of Engineering and Architecture; 2023 Aug 25; Kalasin, Thailand: Kalasin University; p. 258-68.
Vorawongsagul S, Pratumpong P, Pechyen C. Preparation and foaming behavior of poly (lactic acid)/poly (butylene succinate)/cellulose fiber composite for hot cups packaging application. Food Packag Shelf Life. 2021;27:100608.
Zhao L, Huang H, Han Q, Yu Q, Lin P, Huang S, et al. A novel approach to fabricate fully biodegradable poly(butylene succinate) biocomposites using a paper-manufacturing and compression molding method. Composites Part A: Applied Science and Manufacturing. 2020;139:106117.
Sirichalarmkul A, Kaewpirom S. Enhanced biodegradation and processability of biodegradable paGRage from poly(lactic acid)/poly(butylene succinate)/rice-husk green composites. J Appl Polym Sci. 2021;138(27):50652.
Ferdinánd M, Várdai R, Móczó J, Pukánszky B. Poly (lactic acid) reinforced with synthetic polymer fibers: interactions, structure, and properties. Compos Part A-Appl S. 2023;164:107318.
Ruzuqi R. Impact strength analysis of polymer composite materials (PCM) fiber reinforced in the fiberboat application. Material Science Research India. 2020;17(2):170-8.
Badrinath R, Senthilvelan T. Comparative investigation on mechanical properties of banana and sisal reinforced polymer-based composites. Procedia material science. 2014;5:2263-72.
Frollini E, Bartolucci N, Sisti L., Celli A. Biocomposites based on poly(butylene succinate) and curaua: Mechanical and morphological properties. Polymer Testing. 2015;45:168-73.
Frollini E. Bartolucci N. Sisti L. Celli A. Poly(Butylene Succinate) reinforced with different lignocellulosic fibers. Ind Crops Prod. 2013;45:160-9.
Saffian HA, Yamaguchi M, Ariffin H, Abdan K, Kassim NK, Lee SH, et al. Thermal, physical and mechanical properties of poly(butylene succinate)/kenaf core fibers composites reinforced with esterified lignin. Polymers. 2021;13:2359.
Mariatti M, Jannah M, Abu Bakar A, Khalil HA. Properties of banana and pandanus woven fabric reinforced unsaturated polyester composites. J Compos Mater. 2008;42:931-41.
Girijappa YGT, Rangappa M S, Parameswaranpillai J, Siengchin S. Natural fibers as sustainable and renewable resource for development of eco-friendly composites: A comprehensive review. Frontiers in Materials. 2019;6:226.